There are a couple things that can’t be done with a compass and straightedge - squaring a circle, doubling a cube, finding the distance from a point to an ellipse.
Among these is the task of trisecting a given angle. However, despite not being able to be done using classical methods, origami has an algorithm for this construction.
It begins with the angle drawn from the corner (I will, WLOG, refer to the example with the angle in the bottom right corner) of the piece of paper with one ray lying on the paper’s edge and the other ray marked or folded. A fold is made parallel to the edge of the paper with the angle’s ray on it, close to the top. Then, the bottom half of the paper is folded in half.
Next, the point at the intersection of the top fold and the left edge of the paper and the vertex of the angle are folded in such a way that they meet the angle’s ray and the bottom horizontal fold, respectively.
Finally, if you fold from the corner to the point where the diagonal fold intersected the bottom horizontal fold and the point where the angle’s vertex landed, on the bottom horizontal fold, you will get two more lines that perfectly trisect your original angle.
Now, here’s the crucial question: What did using origami add that a straightedge and compass couldn’t? Well, it was that diagonal fold. It added what would amount by straightedge and compass to an infinite amount of information. That fold maps to finding the shared tangent of two parabolas, which requires a cubic equation, which cannot be done using Euclidean methods. Indeed, origami is even more powerful than straightedge and compass.